| Title |
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ja
超微量の炭素同位体比測定による海底熱水・冷湧水溶存気体に関する研究
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en
Stable carbon isotopic studies of volatile components in seafloor venting hydrothermal and cold seep fluids, using CF-IRMS
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| Creator |
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| Accessrights |
open access |
| Subject |
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Other
en
methane
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Other
en
hydrocarbon
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Other
en
CF-IRMS
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Other
en
carbon isotopic composition
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Other
en
hydrothermal and cold seep fluid
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Other
en
carbon monoxide
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Other
en
kinetic isotope frationation
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NDC
450
|
| Description |
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Abstract
en
This paper summarizes stable carbon isotopic studies of hydrocarbons, especially methane, in seafloor venting hydrothermal and cold seep fluids, and their effluent methane-enriched plume in water column. Through highly sensitive isotopic analysis using CF-IRMS, we have discussed origin and/or behavior of hydrocarbons in each system. Major results are as follows: (i) methane in cold seep fluids around Japanese islands mostly microbial origin, (ii) methane emitted from cold seep fluids mostly oxidized anaerobically within sediments just before they emitted into ocean, (iii) methane in hydrothermal plume oxidized aerobically in some extent in the water column. Besides, methane flux and heat flux can be calculated for a methane-enriched fluid venting area from δ13C distribution of methane in hydrothermal plume, by using kinetic isotope fractionation which occurs during partial destruction. Similar approach could be also applicable to study origin and behavior of reactive trace components in atmosphere, such as non-methane hydrocarbons and CO. Preliminary results of such studies are also presented.
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| Publisher |
en
日本地球化学会
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| Date |
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| Language |
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| Resource Type |
journal article |
| Version Type |
VoR |
| Identifier |
HDL
http://hdl.handle.net/2115/44891
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| Journal |
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-
PISSN
0386-4073
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NCID
AN00141280
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ja
地球化学
en
Chikyukagaku (Geochemistry)
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Volume Number36
Issue Number1
Page Start51
Page End63
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| File |
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| Oaidate |
2023-07-26 |
